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This book is thesecond volume of three volume series recording the "Radon Special Semester 2011 on Multiscale Simulation & Analysis in Energy and the Environment" taking place in Linz, Austria, October 3-7, 2011. The volume addresses the common ground in the mathematical and computational procedures required for large-scale inverse problems and data assimilation in forefront applications.It records the achievements of Workshop2 "Large-Scale Inverse Problems and Applications in the Earth Sciences". Itinvolves experts in the theory of inverse problems together with experts working on both theoretical and practical aspects of the techniques by which large inverse problems arise in the earth sciences.